- Jack Black - Jamison Friend
- Aidy Bryant - Anne Severino
- Cedric Yarbrough - Pawn Shop Owner
- John Slattery - William H. Sebastian
- Michael Patrick O'Brien - Young Alexander Krauss
- Heather Hopkins - Hot Teenage Daughter
- Owen Wilson - Father Ra-Shawbard
- Michael Keaton - Bill Doss
- Necar Zadegan - Ra-Sharir
- Connie Chung - Connie Chung
- Taran Killam - Benedict Juniper
- John Mulaney - Simon Sawyer
- James Urbaniak - Howard Pine
- Alex Brightman - Kenny
- Richard Kind - Larry
- Paula Pell - Patty
- Renée Elise Goldsberry - Dee Dee
- Natasha Lyonne - Carla Meola
- Benton Jennings - Rich Snooty Man
- Cate Blanchett - Izabella Barta
- Cate Blanchett - Alice
- Tim Robinson - Young Barnabas Scott
- Maya Rudolph - Anita
- Ty Dolla Sign - Ty Dolla Sign
- Harriet Walter - Edwina
- Trystan Gravelle - Alwyn 'Allie' Lewis-Ifans
- Jonathan Pryce - Owen Teale-Griffith
- John Rhys-Davies - Garth Davies-Gruffudd
- Tom Jones - Bev Turner
- Jamie Demetriou - Benjamin Clay
- Rob Benedict - Larry Fein
- James Thomas Gilbert - Alfred Fein
- Randy Oglesby - Officer #1
- Eric Nenninger - Officer #2
- Sy Richardson - David
- Alexander Skarsgård - Rainer Wolz
- Nicholas Braun - Kevin Butterman
- August Diehl - Dieter Daimler
- Kevin Bishop - Gary Jacks
- Gana Bayarsaikhan - Masho
- Matthias Rimpler - Half-Tone
- Deb Hiett - Narrator (voice)
- Liliane Rovère - Ida Leos
- Ronald Guttman - Pierre Mouland
- Gary Kraus - Howie the Butcher
- Anne Hathaway - Self
- Verona Verbakel - Beatrice Lemutte
- Paola Zampierolo - Young Ida Leos
- David Alade - Lavetrious Kennedy
- David Allen Cress
- Tamsin Rawady
- Matt Pacult
- Erik Kenward
- Alexander Buono
- Andrew Garland
Anne Hathaway hace el papel de Self.
Cate Blanchett interpreta a Alice en la serie.
Owen Wilson interpreta a Father Ra-Shawbard en la serie.
Jonathan Pryce interpreta a Owen Teale-Griffith en la serie.
John Rhys-Davies interpreta a Garth Davies-Gruffudd en la serie.
Fred Armisen hace el papel de Various Characters.
Michael Keaton hace el papel de Bill Doss.
Helen Mirren interpreta a Helen Mirren - Host en la serie.
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