- Andrew Clarke - Simon Templar
- George Rose - Woods
- Christopher Marcantel - Joey
- Holland Taylor - Fran Grogan
- Caitlin Clarke - Lily Palmer / Jessica Daniels
- Liliana Głąbczyńska - Margot Katka
- Raymond Serra - Carmine
- Buddy Ebsen - Buddy Tucker
- James Widdoes - Brian
- Lionel Stander - Sully Carson
- Karen Berger - Greta
- Suzanne Snyder - Andrea
- Christa Denton - Beth
- Tanya Fenmore - Cathy
- Jaclyn Bernstein - Denise
- Warren Munson - Gordon Purcell
- James Naughton - John Dockery
- Kay Lenz - Ray
- Richard Farnsworth - Carl
- Matt Clark - Matt
- Dennis Letts - Dudan
- Carl Weintraub - Dr. Charles Marston
- Gennie James - Sara Marston
- Joseph Mydell - Peter
- Jenifer Landor - Maggie Halston-Cray
- James Eckhouse - David / Max Galpin
- Leslie Jordan - Worm
- Patti Yasutake - Shirley Kajimoto
- Manuel Benitez - Student
- Tim Reid - Self - Host
- Daphne Maxwell Reid - Self - Host
- James Frawley - Jail Cellmate
- Ray Iannicelli - Toy Store Clerk
- Frank Ferrara - Goon
- Kelly Connell - Elevator Man
- Kevin O'Rourke - Detective
- Michael Lombard - Wally Grogan
- Ben Vereen - Pianist in Bar
- Peter Maloney - The Fixer
- Robert LuPone - Jeffery Sinclair
- Kevin Tighe - Insp John Fernack
- Brandon Lee - Johnny Caine
- David Darlow - Kwai Chang Caine
- Miguel Ferrer - Mic
- Paula Kelly - Lt. Lois Poole
- Richard L. Duran - Raul
- Loyda Ramos - Field Hand
- Neil Flynn - LAPD Officer
- Valerie Perrine - Molly
- Brenda Vaccaro - Maxine
- George DelHoyo - Steve Ballinger
- Alex Rocco - Arthur
- Eric Christmas - Edgar
- Meg Wittner - Alice Ballinger
- Hugh Maguire - Jim
- Ted Wass - Mickey
- George Furth - Rip
- Nancy Lenehan - Vivian
- Cleavant Derricks - Marvin
- Florence Stanley - Adele
- Jessie Lawrence Ferguson - Colonel Ntsunge
- Miriam Flynn - Betty
- Richard Hunt - Del
- Jack Burns - Bud Stone
- Lisa Waltz - Holly
- Ron Fassler - Mitchell Bennett
- Marianne Muellerleile - Nurse
- Elya Baskin - Serge
- Bradley Gregg - Russ
- Marsha Waterbury - Dana
- Matt Salinger - James Cabot Barrington
- Robert Beltran - Howard Thunder
- Barbara Bain - Julie Barrington
- Beah Richards - Katherine
- Andrea Marcovicci - Ian Parker / Mandy Keeler
- Ian McShane - Marbury
- Salome Jens - Glenda Davis
- Chelsea Field - Kelsey Baker
- Madeleine Sherwood - Emily Welles
- Bill Morey - Cyrus Welles
- Lee de Broux - Bartender
- Kim Chan - Yuchi
- Tony Wharmby
- Alan Rafkin
- Steve Miner
- David Jackson
- Jeffrey Hornaday
- Peter H. Hunt
- Jeremy Stevens
- Rachel Singer
- Chip Proser
- Gary Markowitz
- Mark Reisman
- Paul De Meo
- Bill Millar
- Bernie Brillstein
- Jim Henson
- Terry Carr
- Margery Simkin
- Susan Shaw
Andrew Clarke interpreta a Simon Templar en la serie.
George Rose hace el papel de Woods.
Christopher Marcantel hace el papel de Joey.
Holland Taylor interpreta a Fran Grogan en la serie.
Caitlin Clarke hace el papel de Lily Palmer / Jessica Daniels.
Liliana Głąbczyńska hace el papel de Margot Katka.
Raymond Serra interpreta a Carmine en la serie.
Buddy Ebsen interpreta a Buddy Tucker en la serie.
Lionel Stander hace el papel de Sully Carson.
Suzanne Snyder interpreta a Andrea en la serie.
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