- Diahann Carroll - Self
- Eddie Foy Jr. - Casey
- David Powers - Self
- Lauren Bacall - Self
- Diana Sands - Self - Wife
- Estelle Winwood - Sarah
- Libby Morris - Self
- Dick Shawn - Paul Benderhof
- Michael Redgrave - Sir Simon Canterville / The Ghost
- Maureen Pryor - Rebecca
- Dick Cavett - Self - Host
- Ricky Nelson - Carlos O'Connor
- Dorothy Stickney - Mrs. Monday
- Katharine Houghton - Bonnie
- Robert Young - Self - Host
- Richard Haydn - Whitey
- Alistair Cooke - Self - Host
- Ingrid Bergman - A Woman
- Arlene Golonka - Mary
- Ben Johnson - Sheriff Barbee
- Rex Everhart - Klein
- Julie Felix - Self
- John Forsythe - Self
- Maurice Chevalier - Self
- Lou Jacobi - Comedian
- Dick Gregory - Self - Civil Rights Marcher
- Charmian Carr - Ella Harkins
- Peter Gennaro - Self
- Reginald Gardiner - Uncle Andrew
- Theodore Bikel - Homer T. Hatch
- Kay Walsh - Greta
- Robert Gerringer - George Blessing
- Anne Bancroft - Virginia
- Arthur Kennedy - Lieutenant Hammond
- Tippy Walker - Virginia Otis
- James Coco - Mr. Zuckerman
- Joe Namath - Quarterback
- Albert Finney - Self
- Peter Noone - David, the Duke of Cheshire
- Lew Ayres - Arthur
- Dina Merrill - Ginny Weldon
- Honor Blackman - Jane & Jill Marriott
- Alan Arkin - Barney Kempinski
- Godfrey Cambridge - Self - Husband
- Brandon De Wilde - Carl Boyer
- Joanie Sommers - Angie
- Bobby Darin - Self
- Ronnie Schell - Self
- Per Oscarsson - Olaf Helton
- Hugh Griffith - Herr Hoffman
- Anthony Perkins - Charles Snell
- Larry Gates - Roscoe Potts
- Count Basie - Self
- John Gielgud - Rich Man
- Moms Mabley - Self - Maid
- Connie Stevens - Flame
- Will Mackenzie - Jerome
- Joan Darling - Peg
- Dana Elcar - Lou Coolidge
- Peter Robbins - Herbert
- Douglas Fairbanks Jr. - Mr. Otis
- Leon Ames - Gray
- Jill Bennett - Frida Holmeier
- Larry Blyden - Todd Bronson
- Danny La Rue - Self
- Alan King - Leo
- Natalie Schafer - Mrs. Otis
- James Broderick - Hal Crady
- Fred Clark - Dean Severance
- Vera Miles - Adele
- Hamilton Dyce - Koorp
- Petula Clark - Self
- Kenneth Connor - Self
- George Kirby - Self
- Hugh Franklin - Howard Boyer
- L.Q. Jones - Deputy
- Tony Randall - Inspector Berry / Geoffrey Judge
- Peter Sellers - Self
- Phyllis Newman - Mary Severance
- Bernard Fox - Jack
- Olivia de Havilland - Ellie Thompson
- Barnard Hughes - Lathrop Hyde
- Redd Foxx - Self - Pool Hustler
- Stuart Whitman - Steve
- Leonardo Cimino - Dino
- Donald O'Connor - Hermes
- Ronnie Corbett - Self
- Jason Robards - Royal Earle Thompson
- Lee Grant - Laura
- Lee Grant - Ruth
- Dustin Hoffman - J.J. Semmons
- Harry Belafonte - Self
- Ruth White - Geraldine
- Carol Lynley - Self
- Laurence Olivier - Self
- Dewey 'Pigmeat' Markham - Self - Comedian
- Carole Mathews - Kay Bartlett
- Conrad Nagel - Mr. Mallory
- Jerry Giesler - Self (archive footage)
- James Mason - Otto Hoffman
- Kenneth Mars - Dr. Pratt
- J. Pat O'Malley - Buttle
- Truman Capote
- Phil Stein
Per Oscarsson hace el papel de Olaf Helton.
Ingrid Bergman interpreta a A Woman en la serie.
Laurence Olivier interpreta a Self en la serie.
James Mason interpreta a Otto Hoffman en la serie.
Larry Gates hace el papel de Roscoe Potts.
Albert Finney hace el papel de Self.
Alan Arkin interpreta a Barney Kempinski en la serie.
Dustin Hoffman hace el papel de J.J. Semmons.
Jason Robards hace el papel de Royal Earle Thompson.
Ricky Nelson interpreta a Carlos O'Connor en la serie.
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